| タイトル | Anthropogenic Emissions of Highly Reactive Volatile Organic Compounds (HRVOCs) Inferred from Oversampling of OMI HCHO Columns |
| 本文（外部サイト） | http://hdl.handle.net/2060/20150000345 |
| 著者（英） | Zhang, Aoxing; Jacob, Daniel; Zhu, Lei; Chance, Kelly; Abad, Gonzalo Gonzalez; Duncan, Bryan; Marais, Eloise; Yoshida, Yasuko; Cohan, Daniel; DeSmedt, Isabelle; Mickley, Loretta |
| 著者所属（英） | NASA Goddard Space Flight Center |
| 発行日 | 2014-09-16 |
| 言語 | eng |
| 内容記述 | Satellite observations of formaldehyde (HCHO) columns provide top-down constraints on emissions of highly reactive volatile organic compounds (HRVOCs). This approach has been used previously to constrain emissions of isoprene from vegetation, but application to US anthropogenic emissions has been stymied by lack of a discernable HCHO signal. Here we show that oversampling of HCHO data from the Ozone Monitoring Instrument (OMI) for 2005 - 2008 enables quantitative detection of urban and industrial plumes in eastern Texas including Houston, Port Arthur, and Dallas-Fort Worth. By spatially integrating the individual urban-industrial HCHO plumes observed by OMI we can constrain the corresponding HCHO-weighted HRVOC emissions. Application to the Houston plume indicates a HCHO source of 260 plus or minus 110 kmol h-1 and implies a factor of 5.5 plus or minus 2.4 underestimate of anthropogenic HRVOC emissions in the US Environmental Protection Agency inventory. With this approach we are able to monitor the trend in HRVOC emissions over the US, in particular from the oil-gas industry, over the past decade. |
| NASA分類 | Earth Resources and Remote Sensing |
| レポートNO | GSFC-E-DAA-TN18604 |
| 権利 | Copyright, Distribution as joint owner in the copyright |
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